安徽旌德-宁国地区大气干湿沉降地球化学特征及评价研究

doi:10.13686/j.cnki.dzyzy.2021.06.013

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Abstract Taking the atmospheric dry and wet deposition in Jingde-Ningguo area of Anhui Province as study object, a total of 24 samples are collected from 6 sites to comparatively analyzes the element content and flux characteristics of atmospheric dry and wet deposition, statistically study the element content and distribution features of dry and wet deposition, and carry out the environmental geochemical evaluation as well. The results show that atmospheric dry and wet deposition elements mainly exist in the form of mineral facies or adsorbed on solid particles, and they are affected by surrounding environment. The high Cd and Se contents in dry deposition have great impact on soil pollution in the study area, the pH values of some wet deposition sampling sites exceed the irrigation water quality criteria, and all sites reach the Grade II surface water environmental quality standard. As to the annual deposition flux density of heavy metal elements, the deposition flux of As is low, Hg, Ni, Pb, Cr, Cu and Cd lower, and Zn higher. The flux of heavy metal elements in dry and wet atmospheric deposition is generally smaller in hilly areas than in towns and industrial/mining areas, mainly affected by coal combustion, exhaust gas emission and human activities. The evaluation results of environmental geochemistry single index and comprehensive index for atmospheric dry and wet deposition are both Grade I.

Key words： atmospheric dry and wet deposition element content deposition flux heavy metal pedogeochemistry Anhui Province

Received: 09 March 2021

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X142

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	Articles by authors
	WU Zheng
	XING Run-hua
	CHEN Fu-rong
	LI Ming-hui
	LIU Chao
	LI Yang

Cite this article:

WU Zheng,XING Run-hua,CHEN Fu-rong等. GEOCHEMISTRY AND EVALUATION OF ATMOSPHERIC DRY AND WET DEPOSITION IN JINGDE-NINGGUO AREA, ANHUI PROVINCE[J]. GEOLOGY AND RESOURCES, 2021, 30(6): 733-739,732.

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http://manu25.magtech.com.cn/Jweb_dzyzy/EN/10.13686/j.cnki.dzyzy.2021.06.013 OR http://manu25.magtech.com.cn/Jweb_dzyzy/EN/Y2021/V30/I6/733

[1]	王梦梦, 原梦云, 苏德纯. 我国大气重金属干湿沉降特征及时空变化规律[J]. 中国环境科学, 2017, 37(11):4085-4096. Wang M M, Yuan M Y, Su D C. Characteristics and spatial-temporal variation of heavy metals in atmospheric dry and wet deposition of China[J]. China Environmental Science, 2017, 37(11):4085-4096.
[2]	秦先燕, 彭苗枝, 焦团理, 等. 基于GIS的环巢湖地区地质环境承载能力评价[J]. 地质与资源, 2020, 29(2):180-186. Qin X Y, Peng M Z, Jiao T L, et al. Assessment of GIS-based geological environment carrying capacity in circum-Chaohu Lake area, Anhui, China[J].Geology and Resources, 2020, 29(2):180-186.
[3]	黄春雷, 宋金秋, 潘卫丰. 浙东沿海某地区大气干湿沉降对土壤重金属元素含量的影响[J]. 地质通报, 2011, 30(9):1434-1441. Huang C L, Song J Q, Pan W F. Impact of dry and wet atmospheric deposition on content of heavy metals in soils along coastal areas of eastern Zhejiang Province[J]. Geological Bulletin of China, 2011, 30(9):1434-1441.
[4]	李延生. 黑龙江省松嫩平原南部大气降尘地球化学特征[J]. 物探与化探, 2011, 35(4):536-540. Li Y S. Geochemical characteristics of atmospheric dust in southern Songnen Plain, Heilongjiang Province[J]. Geophysical & Geochemical Exploration, 2011, 35(4):536-540.
[5]	崔邢涛, 栾文楼, 宋泽峰, 等. 石家庄城市土壤重金属空间分布特征及源解析[J]. 中国地质, 2016, 43(2):683-690. Cui X T, Luan W L, Song Z F, et al. A study of the spatial distribution and source of heavy metals in urban soil in Shijiazhuang City[J]. Geology in China, 2016, 43(2):683-690.
[6]	Kelly J, Thornton I, Simpson P R. Urban geochemistry:A study of the influence of anthropogenic activity on the heavy metal content of soils in traditionally industrial and non-industrial areas of Britain[J]. Applied Geochemistry, 1996, 11(1/2):363-370.
[7]	Lawlor A J, Tipping E. Metals in bulk deposition and surface waters at two upland locations in northern England[J]. Environmental Pollution, 2003, 121(2):153-167.
[8]	汤奇峰, 杨忠芳, 张本仁, 等. 成都经济区As等元素大气干湿沉降通量及来源研究[J]. 地学前缘, 2007, 14(3):213-222. Tang Q F, Yang Z F, Zhang B R, et al. A study of elements flux and sources from atmospheric bulk deposition in the Chengdu economic region[J]. Earth Science Frontiers, 2007, 14(3):213-222.
[9]	庞绪贵, 王晓梅, 代杰瑞, 等. 济南市大气降尘地球化学特征及污染端元研究[J]. 中国地质, 2014, 41(1):285-293. Pang X G, Wang X M, Dai J R, et al. Geochemical characteristics and pollution sources identification of the atmospheric dust-fall in Jinan City[J]. Geology in China, 2014, 41(1):285-293.
[10]	李随民, 栾文楼, 宋泽峰, 等. 河北省南部平原区大气降尘来源及分布特征[J]. 中国地质, 2010, 37(6):1769-1774. Li S M, Luan W L, Song Z F, et al. The distribution and source of atmospheric dust fall in the southern plain of Hebei Province[J]. Geology in China, 2010, 37(6):1769-1774.
[11]	刘国栋, 杨泽, 戴慧敏, 等. 黑龙江省海伦市长发镇土地质量地球化学评价及开发建议[J]. 地质与资源, 2020, 29(6):533-542. Liu G D, Yang Z, Dai H M, et al. Geochemical evaluation of land quality and development suggestion of land in Hailun City, Heilongjiang Province[J]. Geology and Resources, 2020, 29(6):533-542.
[12]	刘鹏, 胡文友, 黄标, 等. 大气沉降对土壤和作物中重金属富集的影响及其研究进展[J]. 土壤学报, 2019, 56(5):1048-1059. Liu P, Hu W Y, Huang B, et al. Advancement in researches on effect of atmospheric deposition on heavy metals accumulation in soils and crops[J]. Acta Pedologica Sinica, 2019, 56(5):1048-1059.
[13]	丛源, 陈岳龙, 杨忠芳, 等. 北京平原区元素的大气干湿沉降通量[J]. 地质通报, 2008, 27(2):257-264. Cong Y, Chen Y L, Yang Z F, et al. Dry and wet atmospheric deposition fluxes of elements in the Plain area of Beijing Municipality, China[J]. Geological Bulletin of China, 2008, 27(2):257-264.
[14]	刘国栋, 张立, 杨泽, 等. 嫩江流域水体及悬浮物重金属元素分布特征及环境指示意义[J]. 地质与资源, 2021, 30(1):53-61. Liu G D, Zhang L, Yang Z, et al. Distribution characteristics of heavy metals in the water and suspended substance of Nenjiang River basin:Environmental implication[J].Geology and Resources, 2021, 30(1):53-61.
[15]	戴彬, 吕建树, 战金成, 等. 山东省典型工业城市土壤重金属来源、空间分布及潜在生态风险评价[J]. 环境科学, 2015, 36(2):507-515. Dai B, Lü J S, Zhan J C, et al. Assessment of sources, spatial distribution and ecological risk of heavy metals in soils in a typical industry-based city of Shandong Province, eastern China[J]. Environmental Science, 2015, 36(2):507-515.
[16]	赵君, 汪月华, 张哲寰. 多目标地球化学调查数据在松嫩平原油气藏远景预测的应用[J].地质与资源, 2020, 29(6):635-640, 626. Zhao J, Wang Y H, Zhang Z H. Application of multi-target geochemical survey data in prospect prediction of the oil-gas reservoirs in Songnen Plain[J]. Geology and Resources, 2020, 29(6):635-640, 626.
[17]	王卫星, 曹淑萍, 李攻科, 等. 津北大气干湿沉降重金属元素通量与评价研究[J]. 环境科学与管理, 2017, 42(5):46-51. Wang W X, Cao S P, Li G K, et al. Sedimentation flux and its evaluation of dry and wet atmospheric deposition of heavy metal elements in North Tianjin[J]. Environmental Science and Management, 2017, 42(5):46-51.
[18]	王琦. 辽东湾北部浅海沉积物铅地球化学评价[J]. 地质与资源, 2019, 28(5):477-481. Wang Q. Geochemical evaluation of lead in the neritic sediments of northern Liaodong Bay[J]. Geology and Resources, 2019, 28(5):477-481.
[19]	崔邢涛, 栾文楼, 李随民, 等. 石家庄市大气降尘重金属元素来源分析[J]. 中国地质, 2012, 39(4):1108-1115. Cui X T, Luan W L, Li S M, et al. An analysis of the sources of heavy metals in atmospheric dust fall of Shijiazhuang city[J]. Geology in China, 2012, 39(4):1108-1115.
[20]	孙雪菲, 张丽霞, 董玉龙, 等. 典型石化工业城市土壤重金属源解析及空间分布模拟[J]. 环境科学, 2021, 42(3):1093-1104. Sun X F, Zhang L X, Dong Y L, et al. Source apportionment and spatial distribution simulation of heavy metals in a typical petrochemical industrial city[J]. Environmental Science, 2021, 42(3):1093-1104.
[21]	Nriagu J O. Changing metal cycles and human health[M]. Berlin:Springer-Verlag, 1984:113-141.
[22]	王增辉. 鲁西南平原区大气干湿沉降元素输入通量及来源浅析:以巨野县为例[J]. 物探与化探,2020, 44(4):839-846. Wang Z H. An analysis of the input flux and source of elements in dry and wet atmospheric deposition of southwest plain of Shandong:A case study of Juye County[J]. Geophysical & Geochemical Exploration, 2020, 44(4):839-846.
[23]	魏明辉, 许江, 李秋燕, 等. 内蒙古鄂伦春旗土壤钼元素的分布特征及主要影响因素[J]. 地质与资源, 2020, 29(6):609-613. Wei M H, Xu J, Li Q Y, et al. Distribution characteristics and main influencing factors of soil molybdenum in Oroqen Qi, Inner Mongolia[J]. Geology and Resources,2020, 29(6):609-613.
[24]	徐宏林, 李定远, 杨军, 等. 湖北省云梦县重金属元素大气干湿沉降通量初探[J]. 资源环境与工程, 2015, 29(6):816-821. Xu H L, Li D Y, Yang J, et al. Preliminary study on flux of atmospheric dry and wet deposition of heavy metal elements in Yunmeng County, Hubei Province[J]. Resources Environment & Engineering, 2015, 29(6):816-821.
[25]	王锐, 张风雷, 徐姝姝, 等. 土壤重金属污染风险筛选值划分方法:以Cd为例[J]. 环境科学, 2019, 40(11):5082-5089. Wang R, Zhang F L, Xu S S, et al. Method of dividing the value of soil heavy metal pollution risk screening:Using Cd as an example[J]. Environmental Science, 2019, 40(11):5082-5089.
[26]	李锋, 刘思源, 李艳, 等. 工业发达城市土壤重金属时空变异与源解析[J]. 环境科学, 2019, 40(2):934-944. Li F, Liu S Y, Li Y, et al. Spatiotemporal variability and source apportionment of soil heavy metals in a industrially developed city[J]. Environmental Science, 2019, 40(2):934-944.
[27]	王硕, 蔡立梅, 王秋爽, 等. 中国城市地表灰尘中重金属的富集状况及空间分布特征[J]. 地理研究, 2018, 37(8):1624-1640. Wang S, Cai L M, Wang Q S, et al. Spatial distribution and accumulation of heavy metals in urban surface dust of China[J]. Geographical Research, 2018, 37(8):1624-1640.
[28]	龚香宜, 祁士华, 吕春玲, 等. 福建省兴化湾大气重金属的干湿沉降[J]. 环境科学研究, 2006, 19(6):31-34. Gong X Y, Qi S H, Lv C L, et al. Atmospheric deposition of heavy metals to Xinghua Bay, Fujian Province[J]. Research of Environmental Sciences, 2006, 19(6):31-34.
[29]	刘娜, 余晔, 马学谦. 西宁市大气污染来源和输送季节特征[J]. 环境科学,2021, 42(3):1268-1279. Liu N, Yu Y, Ma X Q. Seasonal characteristics of air pollutant sources and transport pathways in Xining City[J]. Environmental Science,2021, 42(3):1268-1279.
[30]	Hu W Y, Wang H F, Dong L R, et al. Source identification of heavy metals in peri-urban agricultural soils of southeast China:An integrated approach[J]. Environmental Pollution, 2018, 237:650-661.
[31]	Huang S S, Tu J, Liu H Y, et al. Multivariate analysis of traceelement concentrations in atmospheric deposition in the Yangtze River Delta, East China[J]. Atmospheric Environment, 2009, 43(36):5781-5790.
[32]	严晓瑜, 缑晓辉, 武万里, 等. 银川地区大气颗粒物输送路径及潜在源区分析[J]. 环境科学学报, 2018, 38(5):1727-1738. Yan X Y, Gou X H, Wu W L, et al. Analysis of atmospheric particulate transport path and potential source area in Yinchuan[J]. Acta Scientiae Circumstantiae, 2018, 38(5):1727-1738.
[33]	杨忠平, 卢文喜, 龙玉桥. 长春市城区重金属大气干湿沉降特征[J]. 环境科学研究,2009, 22(1):28-34. Yang Z P, Lu W X, Long Y Q. Atmospheric dry and wet deposition of heavy metals in Changchun City, China[J]. Research of Environmental Sciences, 2009, 22(1):28-34.